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Normalcy: The Normadine 5461
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Normalcy: The Normadine 5461Ion-induced conversion of a magnesium halide perovskite into a halide perovskite.
Interaction between a magnesium and a halide at a metal-halide interface leads to the formation of a Mg-X alloy. This interaction thus provides an important bottom-up approach to the design of new oxide electronic materials. Here, we present the successful formation of cesium lead halide perovskites (PbX3, X = Cl, Br, I) by the exposure of the Mg-Br alloy (Mg0.999Br0.001) to a high-pressure gaseous mixture of PbI2 and X. The Mg-Br alloy is a “mixed-metal” solution, which consists of a dissolved Mg2+ cation and surface-stabilized MgBr2X2+ (X = Cl, Br) complex ions. Exposure to the appropriate gaseous species results in the formation of iodide perovskites in a chemical vapor deposition (CVD) growth mode. The effectiveness of this approach is demonstrated by the preparation of cubic CsPbBr3 and cubic CsPbI3 perovskite crystals. Notably, further ion exchange reactions among the surface MgBr2X2+ complexes are highly effective in converting the Mg-Br alloy into an ordered tetragonal MgI2-Br

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